@Article{TcakaevZRPSDKWSBRABGRH:2020:InAnEu,
author = "Tcakaev, A. and Zabolotnyy, V. B. and Fornari and I and C. and
Ruessmann, P. and Peixoto, T. R. F. and Stier, F. and Dettbarn, M.
and Kagerer, P. and Weschke, E. and Schierle, E. and Bencok, P.
and Rappl, Paulo Henrique de Oliveira and Abramof, Eduardo and
Bentmann, H. and Goering, E. and Reinert, F. and Hinkov, V",
affiliation = "{Universit{\"a}t W{\"u}rzburg} and {Universit{\"a}t
W{\"u}rzburg} and {Universit{\"a}t W{\"u}rzburg} and {Peter
Gr{\"u}nberg Institut and Institute for Advanced Simulation} and
{Universit{\"a}t W{\"u}rzburg} and {Universit{\"a}t
W{\"u}rzburg} and {Universit{\"a}t W{\"u}rzburg} and
{Universit{\"a}t W{\"u}rzburg} and {Helmholtz-Zentrum Berlin
f{\"u}r Materialien und Energie} and {Helmholtz-Zentrum Berlin
f{\"u}r Materialien und Energie} and {Diamond Light Source} and
{Instituto Nacional de Pesquisas Espaciais (INPE)} and {Instituto
Nacional de Pesquisas Espaciais (INPE)} and {Universit{\"a}t
W{\"u}rzburg} and {Max-Planck-Institute for Intelligent Systems}
and {Universit{\"a}t W{\"u}rzburg} and {Universit{\"a}t
W{\"u}rzburg}",
title = "Incipient antiferromagnetism in the Eu-doped topological insulator
Bi2Te3",
journal = "Physical Review B",
year = "2020",
volume = "102",
number = "18",
month = "Nov.",
abstract = "Rare-earth ions typically exhibit larger magnetic moments than
transition-metal ions and thus promise the opening of a wider
exchange gap in the Dirac surface states of topological
insulators. Yet in a recent photoemission study of Eu-doped Bi2Te3
films, the spectra remained gapless down to T = 20 K. Here we
scrutinize whether the conditions for a substantial gap formation
in this system are present by combining spectroscopic and bulk
characterization methods with theoretical calculations. For all
studied Eu doping concentrations, our atomic multiplet analysis of
the M-4,M-5 x-ray absorption and magnetic circular dichroism
spectra reveals a Eu2+ valence and confirms a large magnetic
moment, consistent with a 4f(7) S-8(7/2) ground state. At
temperatures below 10 K, bulk magnetometry indicates the onset of
antiferromagnetic (AFM) ordering. This is in good agreement with
density functional theory, which predicts AFM interactions between
the Eu impurities. Our results support the notion that
antiferromagnetism can coexist with topological surface states in
rare-earth-doped Bi2Te3 and call for spectroscopic studies in the
Kelvin range to look for novel quantum phenomena such as the
quantum anomalous Hall effect.",
doi = "10.1103/PhysRevB.102.184401",
url = "http://dx.doi.org/10.1103/PhysRevB.102.184401",
issn = "1098-0121",
label = "isi 2020-11-16 TcakaevZRPSDKWSBRABGRH:2020:InAnEu",
language = "en",
targetfile = "Incipient antiferromagnetism in the Eu-doped topological insulator
\${_rm Bi}_2{_rm Te}_3\$.pdf",
urlaccessdate = "27 abr. 2024"
}